If you need to remove a users access to an account immediately, the steps below will force a sign-out on all devices signed into with the account.
We highly recommend blocking a users sign-in and reset their password first.
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Login to the Microsoft 365 admin center.
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In the Microsoft 365 admin center, select Users > Active Users > Click on the users Display name you want to sign out of apps and sessions
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For the old admin center: Click OneDrive Settings and click Initiate next to Sign-Out
For the new admin center: click Initiate Sign-out
Resources: